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Understanding the mechanical, surface, and color behavior of oral bioactive prosthetic polymers under biodegradation processes

datacite.subject.fosCiências Médicas::Ciências da Saúde
datacite.subject.sdg03:Saúde de Qualidade
dc.contributor.authorNeves, Cristina B.
dc.contributor.authorCosta, Joana
dc.contributor.authorPortugal, Jaime
dc.contributor.authorBettencourt, Ana F.
dc.date.accessioned2026-03-17T14:20:34Z
dc.date.available2026-03-17T14:20:34Z
dc.date.issued2023-06
dc.description.abstractChanges in the properties of resin-based polymers exposed to the oral environment can emerge when chlorhexidine (CHX) is incorporated to develop bioactive systems for treating denture stomatitis. Three reline resins loaded with CHX were prepared: 2.5 wt% in Kooliner (K), 5 wt% in Ufi Gel Hard (UFI), and Probase Cold (PC). A total of 60 specimens were submitted to physical aging (1000 cycles of thermal fluctuations, 5–55 °C) or chemical aging (28 days of pH fluctuations in artificial saliva, 6 h at pH = 3, 18 h at pH = 7). Knoop microhardness (30 s, 98 mN), 3-point flexural strength (5 mm/min), and surface energy were tested. Color changes (ΔE) were determined using the CIELab system. Data were submitted to non-parametric tests (α = 0.05). After aging, bioactive K and UFI specimens were not different from the controls (resins without CHX) in mechanical and surface properties. Thermally aged CHX-loaded PC specimens showed decreased microhardness and flexural strength but not under adequate levels for function. The color change was observed in all CHX-loaded specimens that underwent chemical aging. The long-term use of CHX bioactive systems based on reline resins generally does not impair removable dentures’ proper mechanical and aesthetic functions.eng
dc.identifier.citationNeves CB, Costa J, Portugal J, Bettencourt AF. Understanding the Mechanical, Surface, and Color Behavior of Oral Bioactive Prosthetic Polymers under Biodegradation Processes. Polymers. 2023; 15(11):2549. https://doi.org/10.3390/polym15112549
dc.identifier.doi10.3390/polym15112549
dc.identifier.issn2073-4360
dc.identifier.urihttp://hdl.handle.net/10400.26/62221
dc.language.isoeng
dc.peerreviewedyes
dc.publisherMDPI
dc.relation.hasversionhttps://doi.org/10.3390/polym15112549
dc.rights.urihttp://creativecommons.org/licenses/by/4.0/
dc.subjectdrug delivery system
dc.subjectacrylic resins
dc.subjectcolor stability
dc.subjectdenture reline
dc.subjectremovable denture
dc.subjectantimicrobial
dc.titleUnderstanding the mechanical, surface, and color behavior of oral bioactive prosthetic polymers under biodegradation processeseng
dc.typecontribution to journal
dspace.entity.typePublication
oaire.citation.issue11
oaire.citation.startPage2549
oaire.citation.titlePolymers
oaire.citation.volume15
oaire.versionhttp://purl.org/coar/version/c_970fb48d4fbd8a85

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